| Schauspieler | Rolle | Synchronsprecher | ||
| Robert Vaughn | Napoleon Solo | Gert Günther Hoffmann | ||
| David McCallum David McCallum | Illya Kuryakin | Eckart Dux Eckart Dux | ||
| Leo G. Carroll | Alexander Waverly | Paul Wagner | ||
| Harry Davis | Alexander Gritzky | Hugo Schrader | ||
| James Doohan | Benjamin Lancer | Siegfried Dornbusch | ||
| Ann Elder | Joanna Sweet | Ingeborg Wellmann | ||
| Bernard Fox | Jordin | Rolf Schult | ||
| Vera Miles | Madame de Sala | Eva Katharina Schultz | ||
| Maurice Evans | Sir Norman Swickert | Eduard Wandrey | ||
| Robert Easton | Texaner | Horst Breitenfeld | ||
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